Excitation Transfer Engineering in Ce-Doped Oxide Crystalline Scintillators by Codoping with Alkali-Earth Ions
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Автор
Auffray, Etiennette
Augulis, Ramunas
Fedorov, Andrei
Dosovitskiy, Georgy
Grigorjeva, Larisa
Gulbinas, Vidmantas
Koschan, Merry
Lucchini, Marco
Melcher, Charles
Nargelas, Saulius
Tamulaitis, Gintautas
Vaitkevicius, Augustas
Zolotarjovs, Aleksejs
Korzhik, Mikhail
Дата
2018Metadata
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Time-resolved spectroscopic study of the photoluminescence response to femtosecond pulse excitation and free carrier absorption at different wavelengths, thermally stimulated luminescence measurements and investigation of differential absorption are applied to amend the available data on excitation transfer in GAGG:Ce scintillators, and an electronic energy-level diagram in this single crystal is suggested to explain the influence of codoping with divalent Mg on luminescence kinetics and light yield. The conclusions are generalized by comparison of the influence of aliovalent doping in garnets (GAGG:Ce) and oxyorthosilicates (LSO:Ce and YSO:Ce). In both cases, the codoping facilitates the energy transfer to radiative Ce3+ centers, while the light yield is increased in the LYSO:Ce system but reduced in GAGG:Ce.